記事
Synthesis of 3,20-disubstituted chlorophyll-a derivatives and reactivity of the substituents
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CiNii Research
Synthesis of 3,20-disubstituted chlorophyll-a derivatives and reactivity of the substituents
資料詳細
要約等：
- Abstract Methyl 20-bromo-pyropheophorbide-a possessing a vinyl group at the 3-position and its analogs having 3-ethyl, 3-(1-hydroxyethyl) and 3-acet...
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デジタル
- 資料種別
- 記事
- 著者標目
- 出版年月日等
- 2013-09
- 出版年（W3CDTF）
- 2013-09
- タイトル（掲載誌）
- Tetrahedron
- 巻号年月日等（掲載誌）
- 69 39
- 掲載巻
- 69
- 掲載号
- 39
- 掲載ページ
- 8412-8421
- 掲載年月日（W3CDTF）
- 2013-09
- ISSN（掲載誌）
- 00404020
- 出版事項（掲載誌）
- Elsevier BV
- 対象利用者
- 一般
- DOI
- 10.1016/j.tet.2013.07.060
- 作成日（W3CDTF）
- 2013-07-24
- 著作権情報
- https://www.elsevier.com/tdm/userlicense/1.0/
- 関連情報（URI）
- 参照
- Transformation of Natural Chlorophyll-<i>a</i> into Chlorophyll-<i>c</i> Analogs Possessing the 17-Acrylate ResidueSynthesis of methyl pyropheophorbide-d derivatives possessing the 3-acyl groups and their electronic absorption spectraPreparation of mono-vinylated and formylated chlorophyll derivatives and their optical propertiesSemi-synthesis and HPLC analysis of (bacterio)chlorophyllides possessing a propionic acid residue at the C17-positionSite-selective C20-fluorinations of chlorophyll-a derivatives using N-fluorobenzenesulfonimide and their optical propertiesSynthesis of deuterated chlorophyll derivatives and their physical propertiesIn vitro reversible dehydration in C3-substituents of zinc chlorophyll analogs by BchF and BchV enzymes: Stereoselectivity and substrate specificity in the dehydrationSynthesis of 20-iodochlorophyll derivatives and their properties including reactivity, electronic absorption, and self-aggregationSynthesis of 7-substituted chlorophyll- a derivatives as chlorophyll- b analogs with specific visible absorption bandsSynthesis of carboxylated chlorophyll derivatives and their activities in dye-sensitized solar cellsSynthesis of zinc 20-ethenylated bacteriochlorophyll-d analogs and their self-aggregation in an aqueous micelle solutionVisible-light-induced hydrogen evolution from water on hybrid photocatalysts consisting of synthetic chlorophyll-a derivatives with a carboxy group in the 20-substituent adsorbed on semiconductors31-Arylation of a chlorophyll-a derivative through Friedel–Crafts alkylationSynthesis of chlorophyll-a derivatives methylated in the 3-vinyl group and their intrinsic site energySynthesis of monovinyl- and divinyl-chlorophyll analogs and their physical propertiesFacile iodination of the vinyl groups in protoporphyrin IX dimethyl ester and subsequent transformation of the iodinated moietiesSynthesis of chlorophyll-a derivatives possessing (un)substituted 131-exo-methylene moiety and their optical propertiesSynthesis of zinc 20-substituted bacteriochlorophyll-d analogs and their self-aggregationSelective synthesis of C32- and C20-monoiodinated chlorophyll derivatives20-(N-Methylpyridiniumyl)ethynylated chlorophyll-a derivative with an intense Qx absorption band at a green to orange regionSynthesis of 20-substituted chlorophyll derivatives with F-ring and optical properties of their less distorted chlorin π-systemsSelf-aggregation of synthetic zinc 3-hydroxymethyl-chlorophyll-<i>a</i> derivatives possessing electron-withdrawing groups at the 20-position in aqueous micelle solutionSynthesis and physical properties of carbonylated chlorophyll derivativesTransformation of carbonyl to vinylidene groups in the π-conjugated peripheral substituent of chlorophyll derivatives by Tebbe reagentSelf‐aggregation of Synthetic Zinc Chlorophyll Derivatives Possessing 3<sup>1</sup>‐Hydroxy or Methoxy Group and 13<sup>1</sup>‐Mono‐ or Dicyanomethylene Moiety in Nonpolar Organic Solvents as Models of Chlorosomal Bacteriochlorophyll‐<i>d</i> AggregatesSynthesis of 20-Deuterated Bacteriochlorophyll-<i>d</i>Homolog and Its 3<sup>1</sup>-Epimerically Controlled Self-aggregationStereoselective self-aggregation of zinc bacteriochlorophyll-d analogs possessing an O-substituted oxime moiety at the 13-positionSubstituted Methylenation at the 13<sup>2</sup>‐Position of a Chlorophyll‐<i>a</i> Derivative <i>via</i> Mixed Aldol Condensation, Optical Properties of the Synthetic Bacteriochlorophyll‐<i>d</i> Analogs, and Self‐aggregation of Their Zinc Complexes<sup>†</sup>Covalent heterodyads of synthetic chlorophyll derivatives linked with linear rigid substituents at the 20-positions constructing photoexcited energy transfer systemsSynthesis of a chlorophyll-a derivative fused with an additional exo-five-membered ring and its optical properties
- 参照
- Modification of 3-Substituents in (Bacterio)Chlorophyll Derivatives to Prepare 3-Ethylated, Methylated, and Unsubstituted (Nickel) Pyropheophorbides and Their Optical PropertiesPhotooxidative cleavage of zinc 20-substituted chlorophyll derivatives: conformationally P-helix-favored formation of regioselectively 19–20 opened linear tetrapyrrolesREVISED METHOD FOR CALCULATION OF GROUP ELECTRONEGATIVITIESConstruction of Chlorosomal Rod Self‐Aggregates in the Solid State on Any Substrates from Synthetic Chlorophyll Derivatives Possessing an Oligomethylene Chain at the 17‐Propionate ResidueMolecular engineering on a chlorophyll derivative, chlorin e6, for significantly improved power conversion efficiency in dye-sensitized solar cellsDouble Helices of a Pyridine-Appended Zinc Chlorophyll DerivativeMolecular Assembly of Zinc Chlorophyll Derivatives by Using Recombinant Light-Harvesting Polypeptides with His-tag and Immobilization on a Gold ElectrodeDicyano-functionalized chlorophyll derivatives with ambipolar characteristic for organic photovoltaicsStereoselective reduction, methylation, and phenylation of the 13-carbonyl group in chlorophyll derivativesSynthesis and epoxide-opening reaction of a 3-oxiranyl-chlorophyll derivativeSynthesis, modification, and optical properties of C3-ethynylated chlorophyll derivativesReduction of vinyl groups in naturally occurring chlorophylls-aRemarkable Regioselective Position-10 Bromination of Bacteriopyropheophorbide-<i>a</i> and Ring-B Reduced Pyropheophorbide-<i>a</i>Supramolecular energy transfer from photoexcited chlorosomal zinc porphyrin self-aggregates to a chlorin or bacteriochlorin monomer as models of main light-harvesting antenna systems in green photosynthetic bacteriaChemosensitive chlorophyll derivatives: optical detection of various amines by synthetic 3-trifluoroacetyl-131-deoxo-pyropheophorbides in solutionA Facile Synthetic Method for Conversion of Chlorophyll-<i>a</i>to Bacteriochlorophyll-<i>c</i>Regioselective Synthesis and Photophysical and Electrochemical Studies of 20‐Substituted Cyanine Dye–Purpurinimide Conjugates: Incorporation of Ni<sup>II</sup> into the Conjugate Enhances its Tumor‐Uptake and Fluorescence‐Imaging AbilityBiomimetic zinc chlorin–poly(4-vinylpyridine) assemblies: doping level dependent emission–absorption regimesRegioselective Bromination Tactics in the de Novo Synthesis of Chlorophyll <i>b</i> Analogues51 Photochemistry of Chlorophylls and Their Synthetic AnalogsSelf-aggregation of synthetic zinc chlorins with a chiral 1-hydroxyethyl group as a model for in vivo epimeric bacteriochlorophyll-c and d aggregatesSinglet and triplet excited state properties of natural chlorophylls and bacteriochlorophyllsSynthesis of Stannyl Porphyrins and Porphyrin Dimers via Stille Coupling and Their <sup>119</sup>Sn NMR and Fluorescence PropertiesThe 17‐Propionate Function of (Bacterio)chlorophylls: Biological Implication of Their Long Esterifying Chains in Photosynthetic Systems<sup>†</sup>Synthetic zinc tetrapyrroles complexing with pyridine as a single axial ligandFORMATION OF OXONIACHLORINS ON PHOTOOXIDATION OF 20‐TRIFLUOROACETOXY‐ AND 20‐CHLORO‐CHLOROPHYLL DERIVATIVES*Photodynamic Tumor Eradication With a Novel Targetable Photosensitizer: Strong Vascular Effects and Dependence on Treatment Repetition <i>Versus</i> PotentiationLinker‐Controlled Energy and Charge Transfer within Chlorophyll TrefoilsStructure Determination of a Bio-Inspired Self-Assembled Light-Harvesting Antenna by Solid-State NMR and Molecular ModelingThe meso substitution of chlorophyll derivatives: direct route for transformation of bacteriopheophorbides d into bacteriopheophorbides c.Synthesis of chlorophyll-a homologs by Wittig and Knoevenagel reactions with methyl pyropheophorbide-dSynthesis of Trifluoromethyl-Porphyrins and -ChlorinsSynthesis of 3/8-carbonylated chlorophyll derivatives and regiodependent reductivity of their carbonyl substituentsPartial syntheses of optically pure methyl bacteriopheophorbides c and d from methyl pheophorbide aPyrroles and related compounds. Part XXIV. Separation and oxidative degradation of chlorophyll derivativesRotational deviation of 3-acetyl group from cyclic tetrapyrrole π-plane in synthetic bacteriochlorophyll-a analogs by 20-substitutionIntramolecular Electron Transfer through the 20-Position of a Chlorophyll <i>a</i> Derivative: An Unexpectedly Efficient Conduit for Charge Transport96 Bacteriochlorophyll Biosynthesis and Assembly in Green Chlorophototrophic Bacteria: Theme and VariationsExtending the limits of natural photosynthesis and implications for technical light harvestingSynthesis and Self-aggregation of Zinc 20-Halogenochlorins as a Model for Bacteriochlorophylls <i>c/d</i>
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