Pd, Pb, Sn, Sb, NbおよびBiに関する熱力学データの整備

Material type: 文書・図像類

Author: Lothenbach, B.ほか

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Publication date: 1999-01

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Note (General)：: This report provides thermodynamic data for predicting concentrations of palladium Pd, lead Pb, tin Sn, antimony Sb, niobium Nb and bismuth Bi in geol...

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Summary, etc.：: This report provides thermodynamic data for predicting concentrations of palladium Pd, lead Pb, tin Sn, antimony Sb, niobium Nb and bismuth Bi in geol...

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Material Type: 文書・図像類
Title: Pd, Pb, Sn, Sb, NbおよびBiに関する熱力学データの整備
Author/Editor: Lothenbach, B.
Ochs, M.
Wanner, H.
油井三和
Author Heading: Lothenbach, B.
Ochs, M.
Wanner, H.
油井三和
Publication Date: 1999-01
Publication Date (W3CDTF): 1999-01
Alternative Title: Thermodynamic Date for the Speciation and Solubility of Pd, Pb, Sn, Sb, Nb, and Bi in Aqueous Solution
Periodical title: JNC TN8400 99-011
Text Language Code: eng
Target Audience: 一般
Note (General): This report provides thermodynamic data for predicting concentrations of palladium Pd, lead Pb, tin Sn, antimony Sb, niobium Nb and bismuth Bi in geologic environments, and contributes to an integration of the JNC chemical thermodynamic database, JNC-TDB (previously PNC-TDB), for the performance analysis of geological isolation system of high-level radioactive wastes. Besides treating hydrolysis in detail, this report focuses on the formation of complexes or compounds with chloride, fluoride, carbonate, nitrate, sulfate and phosphate. Other important inorganic ligands (sulfide for lead and antimony, ammonia for palladium) are also included. In this study, the specific ion interaction theory (SIT) approach is used to extrapolate thermodynamic constants to zero ionic strength at 25$^{\circ}$C.
本報告書では、地層処分システム性能評価のための熱力学データベースJNC-TDB(旧PNC-TDB)整備の一環として実施した、パラジウム(Pd)、鉛(Pb)、スズ(Sn)、アンチモン(Sb)、ニオブ(Nb)およびビスマス(Bi)の6元素に関する熱力学データ整備について報告する。これらの元素に対して、水酸化物錯体の他、塩化物、フッ化物、炭酸、硝酸、硫酸及びリン酸を含む錯体もしくは化合物の生成に焦点を当ててデータ整備を行った。また、鉛およびアンチモンに対しては硫化物錯体、パラジウムに対してはアンモニウム錯体についてもデータ整備を行った。本データ整備においては、SIT(specificioninteractiontheory)アプローチを用いて、25$^{\circ}$C、イオン強度0におけるこれらの錯体もしくは化合物の生成定数を整備した。
Source: /JNC-TN8400-99-011.pdf （fulltext）
https://jopss.jaea.go.jp/pdfdata/JNC-TN8400-99-011.pdf
Access Restrictions: 限定公開
Data Provider (Database): 国立情報学研究所 : 学術機関リポジトリデータベース（IRDB）（機関リポジトリ）
https://irdb.nii.ac.jp
Original Data Provider (Database): 日本原子力研究開発機構 : JOPSS:JAEA Originated Papers Searching System