Atmospheric resuspension of insoluble radioactive cesium-bearing particles found in the difficult-to-return area in Fukushima
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- 資料種別
- 記事
- 著者・編者
- Peng TangKazuyuki KitaYasuhito Igarashi
- 出版年月日等
- 2022-03-14
- 出版年(W3CDTF)
- 2022-03-14
- タイトル(掲載誌)
- Progress in earth and planetary science
- 巻号年月日等(掲載誌)
- 9(17)
- 掲載巻
- 9(17)
- ISSN(掲載誌)
- 2197-4284
- ISSN-L(掲載誌)
- 2197-4284
- 本文の言語コード
- eng
- DOI
- 10.1186/s40645-022-00475-6
- 国立国会図書館永続的識別子
- info:ndljp/pid/12307828
- コレクション(共通)
- コレクション(障害者向け資料:レベル1)
- コレクション(個別)
- 国立国会図書館デジタルコレクション > 電子書籍・電子雑誌 > その他
- 収集根拠
- オンライン資料収集制度
- 受理日(W3CDTF)
- 2022-07-11T20:40:38+09:00
- 保存日(W3CDTF)
- 2022-07-11
- 記録形式(IMT)
- application/pdf
- オンライン閲覧公開範囲
- 国立国会図書館内限定公開
- デジタル化資料送信
- 図書館・個人送信対象外
- 遠隔複写可否(NDL)
- 可
- 掲載誌(国立国会図書館永続的識別子)
- info:ndljp/pid/12307811
- 連携機関・データベース
- 国立国会図書館 : 国立国会図書館デジタルコレクション
- 要約等
- The deposition of insoluble radiocesium-bearing microparticles (CsMPs), which were released from the Fukushima Daiichi Nuclear Power Plant (F1NPP) accident in March 2011, has resulted in the widespread contamination of eastern Japan. Obviously, these deposited insoluble CsMPs may become the secondary contamination sources by atmospheric migration or other environmental transferring process; however, the understanding of the transport mechanism remains non-elucidation, and the relevant evidence has not been directly provided. This study, for the first time, provides the direct evidence for the resuspension of these insoluble CsMPs to the atmosphere from (1) proximity of ¹³⁷Cs radioactivity and resemblance of the morphology and the elemental compositions of CsMPs in the samples of soil and aerosol derived from the same sampling site, (2) the special characteristics of the resuspended CsMPs of which the ratios of Na/Si, K/Si and/or Cs/Si were smaller than those from the initially released CsMPs collected at either long distance or near F1NPP, which can be ascribed to the slowly natural corrosion of CsMPs by the loss of the small amount of soluble contents in CsMPs, and (3) high CsMPs concentration of 10 granules/g in the surface soil of our sampling site and high resuspension frequency of CsMPs in spring when predominant suspended particles were soil dust. Specifically, 15 single CsMPs were successfully isolated from the aerosol filters collected by unmanned high-volume air samplers at a severely polluted area in Fukushima Prefecture, about 25 km away from F1NPP, from January 2015 to September 2019. The mean diameter of these CsMPs was 1.8 ± 0.5 μm, and the average ¹³⁷Cs radioactivity was 0.35 ± 0.23 Bq/granule. The contribution rate of the resuspended CsMPs to the atmospheric radiocesium was estimated from the ratio of ¹³⁷Cs radioactivity of a single CsMP to that of the aerosol filter to be of 23.9 ± 15.3%. There has been no considerable decreasing trend in the annual CsMP resuspension frequency.
- DOI
- 10.1186/s40645-022-00475-6
- オンライン閲覧公開範囲
- インターネット公開
- 著作権情報
- © The Author(s) 2022This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder.
- 関連情報(URI)
- 参照
- Identification, isolation, and characterization of a novel type of Fukushima-derived microparticleRadiocesium-bearing microparticles found in dry deposition fallout samples immediately after the Fukushima nuclear accident in the Kanto region, Japan
- 参照
- Caesium-rich micro-particles: A window into the meltdown events at the Fukushima Daiichi Nuclear Power PlantIsotopic signature and nano-texture of cesium-rich micro-particles: Release of uranium and fission products from the Fukushima Daiichi Nuclear Power PlantNovel method of quantifying cesium-rich microparticles (CsMPs) in the environment from the Fukushima Daiichi nuclear power plantRain-induced bioecological resuspension of radiocaesium in a polluted forest in JapanEffects of Meteorological Conditions on PM2.5 Concentrations in Nagasaki, JapanFirst isolation and analysis of caesium-bearing microparticles from marine samples in the Pacific coastal area near Fukushima PrefectureThe seasonal variations of atmospheric 134,137Cs activity and possible host particles for their resuspension in the contaminated areas of Tsushima and Yamakiya Fukushima Japan福島第一原子力発電所事故の4日後に関東地方で観測された不溶性Cs粒子の生成機構Mass balance and latest fluxes of radiocesium derived from the fukushima accident in the western North Pacific Ocean and coastal regions of JapanUranium Dioxides and Debris Fragments Released to the Environment with Cesium-Rich Microparticles from the Fukushima Daiichi Nuclear Power PlantSoil sampling and analytical strategies for mapping fallout in nuclear emergencies based on the Fukushima Dai-ichi Nuclear Power Plant accidentWeak size dependence of resuspended radiocesium adsorbed on soil particles collected after the Fukushima nuclear accidentDissolution behaviour of radiocaesium-bearing microparticles released from the Fukushima nuclear plantA review of Cs-bearing microparticles in the environment emitted by the Fukushima Dai-ichi Nuclear Power Plant accidentQuantitation of Japanese Cedar Pollen and Radiocesium Adhered to Nonwoven Fabric Masks Worn by the General PopulationFukushima Daiichi reactor source term attribution using cesium isotope ratios from contaminated environmental samplesResuspension of coarse fuel hot particles in the Chernobyl areaLong-term assessment of airborne radiocesium after the Fukushima nuclear accident: Re-suspension from bare soil and forest ecosystemsFirst successful isolation of radioactive particles from soil near the Fukushima Daiichi Nuclear Power PlantEmission of spherical cesium-bearing particles from an early stage of the Fukushima nuclear accidentLand-Surface Contamination by Radionuclides from the Fukushima Daiichi Nuclear Power Plant AccidentAbundance and distribution of radioactive cesium-rich microparticles released from the Fukushima Daiichi Nuclear Power Plant into the environmentDiscovery of Radiocesium-bearing Particles in Masks Worn by Members of the Public in Fukushima in Spring 2013Resuspension and redistribution of radionuclides during grassland and forest fires in the Chernobyl exclusion zone: part I. Fire experimentsAtmospheric effects of Fukushima nuclear accident: A review from a sight of atmospheric monitoringControlled Wind Tunnel Experiments for Particle Bounceoff and ResuspensionUse of a size-resolved 1-D resuspension scheme to evaluate resuspended radioactive material associated with mineral dust particles from the ground surfaceTracking the Fukushima RadionuclidesThe Fukushima nuclear power plant accidentRe-entrainment of the Chernobyl-Derived Radionuclides in Air: Experimental Data and ModelingWind tunnel experiments on the resuspension of particulate materialDetection of Uranium and Chemical State Analysis of Individual Radioactive Microparticles Emitted from the Fukushima Nuclear Accident Using Multiple Synchrotron Radiation X-ray AnalysesSulfate Aerosol as a Potential Transport Medium of Radiocesium from the Fukushima Nuclear AccidentDepth profiles of radioactive cesium in soil using a scraper plate over a wide area surrounding the Fukushima Dai-ichi Nuclear Power Plant, JapanFungal spore involvement in the resuspension of radiocaesium in summerParticulate plutonium released from the Fukushima Daiichi meltdownsDistribution and retention of Cs radioisotopes in soil affected by Fukushima nuclear plant accidentTemporal variation of monthly 137Cs deposition observed in Japan: Effects of the Fukushima Daiichi nuclear power plant accidentPerspective on the Biological Impact of Exposure to Radioactive Cesium-Bearing Insoluble ParticlesAssessment of DNA Damage Induction in Farm Animals After the FNPP AccidentComparison of the Chernobyl and Fukushima nuclear accidents: A review of the environmental impactsAnnual and Weekly Cycles of Radioactivity Concentration Observed in Fukushima CitySecondary radiocesium contamination of agricultural products by resuspended matterReactor environment during the Fukushima nuclear accident inferred from radiocaesium-bearing microparticlesIsotopic ratios of uranium and caesium in spherical radioactive caesium-bearing microparticles derived from the Fukushima Dai-ichi Nuclear Power PlantInternal exposure risk due to radiocesium and the consuming behaviour of local foodstuffs among pregnant women in Minamisoma City near the Fukushima nuclear power plant: a retrospective observational studyRadiocesium and radioiodine in soil particles agitated by agricultural practices: Field observation after the Fukushima nuclear accidentActivity of <sup>90</sup>Sr in Fallout Particles Collected in the Difficult-to-Return Zone around the Fukushima Daiichi Nuclear Power PlantEffectiveness of landscape decontamination following the Fukushima nuclear accident: a reviewEVALUATIONS OF INVENTORY AND ACTIVITY CONCENTRATION OF RADIOCESIUM IN SOIL AT A RESIDENTIAL HOUSE 3 YEARS AFTER THE FUKUSHIMA NUCLEAR ACCIDENTTemporal variation of post-accident atmospheric 137 Cs in an evacuated area of Fukushima Prefecture: Size-dependent behaviors of 137 Cs-bearing particlesPhysical properties, structure, and shape of radioactive Cs from the Fukushima Daiichi Nuclear Power Plant accident derived from soil, bamboo and shiitake mushroom measurementsFukushima Daiichi Nuclear Plant accident: Atmospheric and oceanic impacts over the five yearsVertical profiles of Iodine-131 and Cesium-137 in soils in Fukushima Prefecture related to the Fukushima Daiichi Nuclear Power Station AccidentCharacterization of hydrocarbons in aerosols and investigation of biogenic sources as a carrier of radiocesium isotopesAnalysis of two forms of radioactive particles emitted during the early stages of the Fukushima Dai-ichi Nuclear Power Station accidentDiscovery of radiocesium-bearing microparticles in river water and their influence on the solid-water distribution coefficient (Kd) of radiocesium in the Kuchiboso River in Fukushimaつくばと飯舘における福島第一原発事故由来の大気中放射性セシウム濃度の変化と高濃度現象の要因Atmospheric radioactivity over Tsukuba, Japan : a summary of three years of observations after the FDNPP accident
- 連携機関・データベース
- 国立情報学研究所 : CiNii Research
- 提供元機関・データベース
- 学術機関リポジトリデータベース雑誌記事索引データベースCrossref科学研究費助成事業データベース科学研究費助成事業データベースCrossrefCrossref
- 書誌ID(NDLBibID)
- 12307828