多核金属錯体の核間π共役相互作用と酸化還元電位

Material type: 文書・図像類

Author: 陳, 競鳶ほか

Publisher: 日本ポーラログラフ学会

Publication date: 2000

Material Format: Digital

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Note (General)：: Polynuclear metal ctomplexes of which redox sites are connected with π-conjugated ligands take a number of mixed valence states. They exhibit several ...

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Material Type: 文書・図像類
Title: 多核金属錯体の核間π共役相互作用と酸化還元電位
Author/Editor: 陳, 競鳶
青木, 幸一
CHEN, Jingyuan
AOKI, Koichi
Author Heading: 陳, 競鳶
青木, 幸一
CHEN, Jingyuan
AOKI, Koichi
Publication, Distribution, etc.: 日本ポーラログラフ学会
Publication Date: 2000
Publication Date (W3CDTF): 2000
Alternative Title: Redox potentials of polynuclear metal complexes by π-conjugated metal-interaction
Periodical title: Review of Polarography
No. or year of volume/issue: 46
Volume: 46
Pages: 87-104
Text Language Code: jpn
Subject Heading: polynuclear metal complexes
conjugated metal-interaction
Target Audience: 一般
Note (General): Polynuclear metal ctomplexes of which redox sites are connected with π-conjugated ligands take a number of mixed valence states. They exhibit several redox potentials owing to interaction between redox centers through the π-conjugated bridges. Questions arise about the definition of the interaction, a relation between the number of nuclei and the number of redox potentials, and a relationship between redox potentials and geometry of the complexes. This paper answers these questions thermodynamically as well as quantum mechanically. The interaction energy in this paper is defined as a pair energy between a reduced and an oxidized sites. Even this simplest definition generates complicated redox behaviors because of formation of various isomers when the number metal centers increases.
Access Restrictions: 限定公開
Data Provider (Database): 国立情報学研究所 : 学術機関リポジトリデータベース（IRDB）（機関リポジトリ）
https://irdb.nii.ac.jp
Original Data Provider (Database): 福井大学 : 福井大学学術機関リポジトリ